Answer with explanation:
Number of faces of this unique Die = 10
Theoretical probability of rolling a 3

Now, the die is rolled 20, times.
Number of times, the rolls results in 3= 4
Probability of rolling '3'

but, if you roll the die twenty times, Probability of rolling '3' should be

When we want, theoretical probability and experimental probability,match each other, the number of trials should be large enough to get closer and better results.
The adjustment can Jonas make to his experiment so the theoretical and experimental probabilities are likely to be closer:
D: He can increase the number of trials.